Abstract
The infrared-diode-laser probe technique is a powerful new method for studying molecular-dynamic processes because of its combination of the very high spectral resolution of the diode laser (0.0003 cm−1) and its temporal resolution of 100 ns. Using this technique, we measured, for the first time to our knowledge, the transient changes of the vibrational mode v2 of NH3 caused by collisions with excited NO2.
© 1993 Optical Society of America
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